Topological Optical Chirality Dichroism
Abstract
We report on a universal topological dichroism of chiral three-dimensional systems in response to the chirality of light. We show that chiral topological invariants result in integer-quantized dichroic excitation rate differences. Moreover, we demonstrate that such topological effects arise more generally from coupling optical chirality to higher tensor Berry curvatures and Dixmier-Douady invariants of quantum states, including Hopf indices. We finally propose an experimental setup that leverages superchiral light as a smoking-gun probe of chiral band topologies in three-dimensional materials. Our findings establish an optical route for probing to date unobserved chiral electronic band topologies.
Source: arXiv:2603.28752v1 - http://arxiv.org/abs/2603.28752v1 PDF: https://arxiv.org/pdf/2603.28752v1 Original Link: http://arxiv.org/abs/2603.28752v1